Plasmonic control of radiative properties of semiconductor quantum dots coupled to plasmonic ring cavities

Aliaksandra Rakovich, Pablo Albella, Stefan A. Maier

Research output: Contribution to journalReview articlepeer-review

35 Citations (Scopus)

Abstract

In recent years, a lot of effort has been made to achieve controlled delivery of target particles to the hotspots of plasmonic nanoantennas, in order to probe and/or exploit the extremely large field enhancements produced by such structures. While in many cases such high fields are advantageous, there are instances where they should be avoided. In this work, we consider the implications of using the standard nanoantenna geometries when colloidal quantum dots are employed as target entities. We show that in this case, and for various reasons, dimer antennas are not the optimum choice. Plasmonic ring cavities are a better option despite low field enhancements, as they allow collective coupling of many quantum dots in a reproducible and predictable manner. In cases where larger field enhancements are required, or for larger quantum dots, nonconcentric ring-disk cavities can be employed instead.
Original languageEnglish
Article number10.1021/nn506433e
Pages (from-to)2648-2658
Number of pages11
JournalACS Nano
Volume9
Issue number3
Early online date27 Jan 2015
DOIs
Publication statusPublished - 24 Mar 2015

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